锁显 求是科创学者
博士,研究员,“浙大科创百人”
职务:分子智造所 PI
研究方向:吸附分离、多孔聚合物、智能合成表征、高纯电子化学品、碳捕集
邮箱:xiansuo@zju.edu.cn
地址:杭州市萧山区建设三路733号浙江大学杭州国际科创中心
个人简介:
锁显,浙江大学杭州国际科创中心百人计划研究员,国家优秀青年基金获得者,入选杭州市西湖明珠工程特殊支持计划。2013年获厦门大学学士学位,2018年获浙江大学博士学位,之后入职浙江大学进行博士后研究,2019-2021年期间赴美国田纳西大学从事博士后研究,2022年入职浙江大学杭州国际科创中心。主要从事高纯电子化学品分离纯化、痕量杂质脱除、碳捕集与吸附分离材料智能筛选等方向的研究,获中国化工学会科学技术奖基础研究成果一等奖、2024 ISPT-IACC Future Star Award、2023 IChemE & CCST Young Investigator Award、“离子液体与绿色过程”新秀奖(2023)、腾讯碳寻计划TOP30(2023)等奖励。共发表论文50余篇,其中以一作/通讯作者(含共同)在Adv. Mater.(2篇)、J. Am. Chem. Soc.、Angew. Chem. Int. Ed.(2篇)、Adv. Funct. Mater.、CCS Chem.等期刊发表20余篇,授权中国发明专利4项,主持面上项目、青年项目、国家基金国家重大仪器研制项目课题、国家重点研发计划项目子课题、浙江省自然科学基金重大项目课题等项目10项。
研究成果:
1. 针对炔烃烯烃分离和痕量二氧化硫深度脱除需求,设计高选择性离子超微孔聚合物。
2. 围绕碳捕集和碳转化的需求,设计新型功能化介质,避免副反应和实现吸收焓的调控。
3. 针对结构相似天然活性物质分离需求,设计高选择性的离子功能化多孔聚合物。
代表性论文:
1. Xian Suo, Xili Cui, Lifeng Yang, Nan Xu, Yuqi Huang, Yi He, Sheng Dai, Huabin Xing*, Synthesis of ionic ultramicroporous polymers for selective separation of acetylene from ethylene. Adv. Mater. 2020, 32 (29), 1907601.
2. Xian Suo, Ying Yu, Siheng Qian, Lin Zhou, Xili Cui*, Huabin Xing, Tailoring the pore size and chemistry of ionic ultramicroporous polymers for trace sulfur dioxide capture with high capacity and selectivity. Angew. Chem. Int. Ed.2021, 60, 6986-6991.
3. Xian Suo, Yuqing Fu, Chi-Linh Do-Thanh, Li-Qi Qiu, De-en Jiang, Shannon M. Mahurin, Zhenzhen Yang*, Sheng Dai*, CO2 chemisorption behavior in conjugated carbanion-derived ionic liquids via carboxylic acid formation. J. Am. Chem. Soc. 2022, 144 (47), 21658-21663.
4. Xian Suo#, Fengtao Zhang#, Zhenzhen Yang*, Hao Chen, Tao Wang, Zongyu Wang, Takeshi Kobayashi, Chi-Linh Do-Thanh, Dmitry Maltsev, Zhimin Liu*, Sheng Dai*, Highly perfluorinated covalent triazine frameworks derived from a low-temperature ionothermal approach towards enhanced CO2 electroreduction. Angew. Chem. Int. Ed. 2021, 60 (49), 25688-25694.
5. Hanqian Pan, Xian Suo*, Zhenglu Yang, Lifeng Yang, Xili Cui, Huabin Xing*, Engineering the pore structure and functionality of ionic porous polymers for separating acetylene over carbon dioxide. Adv. Funct. Mater. 2023, 33, 2214887.
6.Yuqi Ke, Yi Chen, Zhenkang Li, Wanmei Li, Xili Cui, Pengfei Zhang*, Xian Suo*, Huabin Xing. Highly efficient deterpenation of essential oils in ionic porous organic polymers through multiple hydrogen-bonding interactions. Chem. Eng. J2024, 481, 148509.
7. Sen Chen#, Shicheng Huang#, Zhenglu Yang, Xian Suo*, Huabin Xing, and Xili Cui*. Precise construction of nitrogen-enriched porous ionic polymers as highly efficient sulfur dioxide adsorbent. Small 2024, 20, 2400746.
8. Hanqian Pan, Junqin Zhao, Lifeng Yang, Xian Suo*, Xili Cui, Huabin Xing*. Modulating pore microenvironment in a robust ionic porous polymer for efffcient propyne/propylene separation. Chem. Eng. Sci. 2024, 298, 120413.
9. Xian Suo#, Hanqian Pan#, Liyuan Chen, Xili Cui, Huabin Xing*, Control of functionalized pore environment in robust ionic ultramicroporous polymers for efficient removal of trace propyne from propylene. ACS Appl. Mater. Interfaces 2021, 13 (36), 42706-42714.
10. Hanqian Pan, Xian Suo*, Zhenglu Yang, Liyuan Chen, Xili Cui, Huabin Xing*, Selective separation of acetylene from ethylene with branched ionic ultramicroporous polymer. Sep. Purif. Technol. 2021, 279, 119728.
11. Hao Chen#, Xian Suo#, Zhenzhen Yang*, Sheng Dai*, Graphitic aza-fused π-conjugated networks: construction, engineering, and task-specific applications. Adv. Mater. 2022, 34, 2107947.
12. Xian Suo#, Fengtao Zhang#, Zhenzhen Yang*, Lu Wang, Ming Lei, James A. Gaugler, Meijia Li, Juntian Fan, Bishnu P. Thapaliya, Ilja Popovs, Alexander S. Ivanov, Leighanne C. Gallington, De-en Jiang, Zhimin Liu*, Sheng Dai*. Electrochemical CO2-to-ethylene conversion on metal-free covalent quinazoline network-derived electrodes. Chem Catal. 2023, 3 (2), 100506.
13. Xian Suo, Yuqing Fu, Juntian Fan, Chi-Linh Do-Thanh, De-en Jiang, Shannon M. Mahurin, Zhenzhen Yang*, Sheng Dai*. Expeditious coordination-driven construction of hierarchically nanoporous barium salts. CCS Chem. 2023, 5, 1517-1525.
14. Hanqian Pan, Cong Yu, Xian Suo,* Lifeng Yang, Xili Cui and Huabin Xing*. Emerging porous materials for carbon dioxide adsorptive capture: progress and challenges. Mater. Chem. Front. 2023, 7, 6463-6482.
15. Penghui Zhang#, Pengyuan Yin#, Lifeng Yang, Xili Cui, Huabin Xing, Xian Suo*. Recent advances and challenges in ionic materials for post-combustion carbon capture, Carbon Capture Science & Technology 2024, 11, 100180.
16.Pengyuan Yin, Yechen Liu, Chenyuan Zhang, Zhenglu Yang, Penghui Zhang, Xian Suo*, Lifeng Yang, Huabin Xing, Xili Cui*. Precise pore structure regulation of an oxalate-functionalized metal–organic framework for efficient carbon dioxide sieving with high capacity, Industrial & Engineering Chemistry Research 2024, DOI: 10.1021/acs.iecr.4c03299.
17.Xian Suo, Zhenzhen Yang*, Yuqing Fu, Chi-Linh Do-Thanh, Dmitry Maltsev, Huimin Luo, Shannon M. Mahurin, De-en Jiang, Huabin Xing*, Sheng Dai*, New-generation carbon-capture ionic liquids regulated by metal-ion coordination. ChemSusChem 2022, 15, e202102136.
18.Xian Suo, Zhenzhen Yang*, Yuqing Fu, Chi-Linh Do-Thanh, Dmitry Maltsev, Huimin Luo, Shannon M. Mahurin, De-en Jiang, Huabin Xing*, Sheng Dai*, CO2 chemisorption behavior of coordination-derived phenolate sorbents. ChemSusChem 2021, 14, 2854-2859.
19. Xian Suo#, Yuqi Huang#, Zhenkang Li, Hanqian Pan, Xili Cui, Huabin Xing*, Construction of anion-functionalized hypercrosslinked ionic porous polymers for efficient separation of bioactive molecules. Sci. China Mater. 2022, 65 (4), 1068-1075.
20. 陈森,殷鹏远,杨证禄,莫一鸣,崔希利,锁显*,邢华斌,功能固体材料智能合成研究进展. 化工进展,2023, 42, 3340-3348.
21. Xian Suo, Ling Xia, Qiwei Yang, Zhiguo Zhang, Zongbi Bao, Qilong Ren, Yiwen Yang, Huabin Xing*, Synthesis of anion-functionalized mesoporous poly(ionic liquid)s via a microphase separation-hypercrosslinking strategy: highly efficient adsorbents for bioactive molecules. J. Mater. Chem. A 2017, 5 (27), 14114-14123.
科研项目:
1. 国家自然科学基金面上项目,基于顶替再生的强吸附气体分离过程及多组分竞争吸附研究,2023/01-2026/12,主持;
2. 国家自然科学基金重大科研仪器研制项目,智能化、高通量吸附剂制备评测仪器,2023/01-2027/12,主持课题;
3. 国家自然科学基金青年项目,基于超支化离子液体的超微孔聚合物的制备及乙炔乙烯分离性能研究,2020/01-2022/12,主持;
4. 国家重点研发计划项目,烯烃烷烃吸附分离材料及应用基础(课题3),2022/11-2025/10,主持子课题;
5. 浙江省科技计划“尖兵”项目,高纯化学试剂的研发与产业示范,2023/01-2025/12,主持子课题;
6. 浙江省自然科学基金重大项目,结构相似碳氢化合物分离材料构建与分离强化机制研究,2024/01-2026/12,合作单位;
7. 杭州铂时生物科技有限公司合作项目,原位沉淀高黏附助剂研发,2022/06-2024/06,主持。
专利:
1.一种超支化离子多孔有机聚合物材料及其制备方法和应用,ZL202211612712.X,锁显、潘罕骞、邢华斌、崔希利、陈丽媛;
2.一类超微孔离子聚合物材料及其制备方法和应用, ZL202010235304.1, 20210305,邢华斌、锁显、崔希利;
3.一种混合生育酚的分离方法及一种多孔聚离子液体材料及其制备方法, 20201215,ZL201710391953.9,邢华斌、锁显、杨启炜、杨亦文、任其龙、张治国;
4. 一种利用聚离子液体从混合生育酚中分离单个生育酚的方法, 20201215,ZL201710395583.6邢华斌、锁显、杨启炜、杨亦文、任其龙、鲍宗必。
荣誉及奖励:
1. 中国化工学会科学技术奖基础研究成果一等奖(2024,3/8)
2. 2024 ISPT-IACC Future Star Award(2024)
3. 2023 IChemE & CCST Young Investigator Award(2023)
4. 腾讯碳寻计划TOP30(2023,2/4)
5. “离子液体与绿色过程”新秀奖(2023)
课题组主页:
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浙江大学个人主页链接:锁显-个人主页
(https://person.zju.edu.cn/suoxian)